Journal of Animal and Veterinary Advances · 2009 · 20 citations · 0 references
Stringent mitigation measures have reduced wintertime fine particulate matter (PM<sub>2.5</sub>) concentrations by 42.2% from 2013 to 2018 in the Beijing-Tianjin-Hebei (BTH) region, but severe PM pollution still frequently engulfs the region. The observed nitrate aerosols have not exhibited a significant decreasing trend and constituted a major fraction (about 20%) of the total PM<sub>2.5</sub>, although the surface-measured NO<sub>2</sub> concentration has decreased by over 20%. The contributions of nitrogen oxides (NO<sub>X</sub>) emissions mitigation to the nitrate and PM<sub>2.5</sub> concentrations and how to alleviate nitrate aerosols efficiently under the current situation still remains elusive. The WRF-Chem model simulations of a persistent and heavy PM pollution episode in January 2019 in the BTH reveal that NO<sub>X</sub> emissions mitigation does not help lower wintertime nitrate and PM<sub>2.5</sub> concentrations under current conditions in the BTH. A 50% reduction in NO<sub>X</sub> emissions only decreases nitrate mass by 10.3% but increases PM<sub>2.5</sub> concentrations by 3.2%, because the substantial O<sub>3</sub> increase induced by NO<sub>X</sub> mitigation offsets the HNO<sub>3</sub> loss and enhances sulfate and secondary organic aerosols formation. Our results are further consolidated by the occurrence of severe PM pollution in the BTH during the COVID-19 outbreak, with a significant reduction in NO<sub>2</sub> concentration. Mitigation of NH<sub>3</sub> emissions constitutes the priority measure to effectively lower the nitrate and PM<sub>2.5</sub> concentrations in the BTH under current conditions, with 35.5% and 12.7% decrease, respectively, when NH<sub>3</sub> emissions are reduced by 50%.