Physical Review A · 2015 · 16 citations · 30 references
Natural SciencesPhysicsCondensed Matter PhysicsOpticsSpectroscopyNonlinear OpticsOptical SpectroscopyAbsorption Line SpectroscopyExcited-state AbsorptionExcited-state DynamicsExcited-state RelaxationExperimental Results InterpretationMagneto-optic EffectsMagneto-optical EffectsMagneto-optical Properties
We present experimental and numerical studies of nonlinear magneto-optical rotation (NMOR) in rubidium vapor excited with resonant light tuned to the $5{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}\ensuremath{\rightarrow}6{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{1/2}$ absorption line (421 nm). Contrary to the experiments performed to date on the strong ${D}_{1}$ or ${D}_{2}$ lines, in this case, the spontaneous decay of the excited state $6{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{1/2}$ may occur via multiple intermediate states, affecting the dynamics, magnitude, and other characteristics of NMOR. Comparing the experimental results with the results of modeling based on Auzinsh et al. [Phys. Rev. A 80, 053406 (2009)], we demonstrate that despite the complexity of the structure, NMOR can be adequately described with a model, where only a single excited-state relaxation rate is used.
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