Advanced Functional Materials · 2018 · 1.5K citations · 275 references
EngineeringMaterials EngineeringMaterials ScienceElectronic MaterialsSemiconductor DevicesSemiconductor MaterialsInfrared DetectorsOptical Properties Of SemiconductorsOptical Properties Of SolidsOptoelectronic MaterialsSemiconductor Device MaterialsTwo-dimensional SemiconductorsBandwidthBlack PhosphorusHeterostructuresHexagonal Boron NitrideOptoelectronic PropertiesSpectrum DetectionTransition Metal DichalcogenidesTwo-dimensional Material Photodetectors
2D material photodetectors have attracted extensive research because their unique structures and superior electronic and optoelectronic properties enable a wide bandgap range and hundreds of reported devices. This review surveys 2D‑material photodetectors across the ultraviolet to infrared spectrum. The authors outline key detection mechanisms, figure‑of‑merit metrics, recent advances, and initial applications of 2D‑material photodetectors. State‑of‑the‑art 2D photodetectors achieve broadband detection, ultrahigh responsivity and sensitivity, rapid response, high bandwidth, and polarization sensitivity, while the review identifies challenges and future directions for high‑performance device design.
Abstract 2D material based photodetectors have attracted many research projects due to their unique structures and excellent electronic and optoelectronic properties. These 2D materials, including semimetallic graphene, semiconducting black phosphorus, transition metal dichalcogenides, insulating hexagonal boron nitride, and their various heterostructures, show a wide distribution in bandgap values. To date, hundreds of photodetectors based on 2D materials have been reported. Here, a review of photodetectors based on 2D materials covering the detection spectrum from ultraviolet to infrared is presented. First, a brief insight into the detection mechanisms of 2D material photodetectors as well as introducing the figure‐of‐merits which are key factors for a reasonable comparison between different photodetectors is provided. Then, the recent progress on 2D material based photodetectors is reviewed. Particularly, the excellent performances such as broadband spectrum detection, ultrahigh photoresponsivity and sensitivity, fast response speed and high bandwidth, polarization‐sensitive detection are pointed out on the basis of the state‐of‐the‐art 2D photodetectors. Initial applications based on 2D material photodetectors are mentioned. Finally, an outlook is delivered, the challenges and future directions are discussed, and general advice for designing and realizing novel high‐performance photodetectors is given to provide a guideline for the future development of this fast‐developing field.
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