Review of Scientific Instruments · 2012 · 164 citations · 46 references
Natural SciencesChemistryPhysicsAnalytical ChemistryOpticsSpectroscopyTime-resolved SpectroscopyX-ray Data AnalysisX-ray OpticsX-ray SpectroscopyEnergy Dispersive X-ray SpectroscopyFree-electron LasersRadiation DamageRaman ScatteringResonant Inelastic X-ray ScatteringSingle ShotTime-resolved X-ray SpectroscopyX-ray Emission Spectroscopy
A multi-crystal wavelength dispersive hard x-ray spectrometer with high-energy resolution and large solid angle collection is described. The instrument is specifically designed for time-resolved applications of x-ray emission spectroscopy (XES) and x-ray Raman scattering (XRS) at X-ray Free Electron Lasers (XFEL) and synchrotron radiation facilities. It also simplifies resonant inelastic x-ray scattering (RIXS) studies of the whole 2d RIXS plane. The spectrometer is based on the Von Hamos geometry. This dispersive setup enables an XES or XRS spectrum to be measured in a single-shot mode, overcoming the scanning needs of the Rowland circle spectrometers. In conjunction with the XFEL temporal profile and high-flux, it is a powerful tool for studying the dynamics of time-dependent systems. Photo-induced processes and fast catalytic reaction kinetics, ranging from femtoseconds to milliseconds, will be resolvable in a wide array of systems circumventing radiation damage.
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First lasing and operation of an ångstrom-wavelength free-electron laser
P. Emma, R. Akre, John Arthur et al. · Nature Photonics · 2010 · 3.1K citations
Natural Sciences, Physics, Optics +10
Resonant inelastic x-ray scattering studies of elementary excitations
L. J. P. Ament, Michel van Veenendaal, Thomas Devereaux et al. · Reviews of Modern Physics · 2011 · 1.3K citations · Full text