ACS Applied Materials & Interfaces · 2023 · 25 citations · 41 references
Natural SciencesMaterials EngineeringMaterials ScienceOptical MaterialsOptoelectronicsSemiconductor MaterialsLight-emitting DiodesLuminescent MaterialsOptoelectronic DevicesOptoelectronic MaterialsPerovskite MaterialsSemiconductor NanomaterialsBlue Light-emitting DiodesElectroluminescenceExternal Quantum EfficiencyLight-emitting DevicesPerovskite Light-emitting DiodesPhotoluminescencePhotoluminescence Quantum YieldQuantum Efficiency
The performance of the blue perovskite light-emitting diodes (PeLEDs) is limited by the low photoluminescence quantum yields (PLQYs) and the unstable emission centers. In this work, we incorporate sodium bromide and acesulfame potassium into a quasi-2D perovskite to control the dimension distribution and promote the PLQYs. Benefiting from the efficient energy cascade channel and passivation, the sky-blue PeLED has an external quantum efficiency of 9.7% and no shift of the electroluminescence center under operation voltages from 4 to 8 V. Moreover, the half lifetime of the devices reaches 325 s, 3.3 times that of control devices without additives. This work provides new insights into enhancing the performance of blue PeLEDs.
41
Perovskite light-emitting diodes based on spontaneously formed submicrometre-scale structures
Yu Cao, Nana Wang, He Tian et al. · Nature · 2018 · 2K citations