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Weakened d–p orbital hybridization in<i>in situ</i>reconstructed Ru/β-Co(OH)<sub>2</sub>heterointerfaces for accelerated ammonia electrosynthesis from nitrates
180
Citations
60
References
2023
Year
EngineeringElectron-deficient Ru SitesOrganometallic ElectrochemistryChemistryAmmonia IntermediatesChemical EngineeringD–p Orbital HybridizationMaterials ScienceInorganic ChemistryMolecular ElectrochemistrySurface ElectrochemistryCatalysisQuantum ChemistryFurther FacilitateAmmonia ElectrosynthesisElectrochemistryOxygen Reduction ReactionNatural SciencesApplied PhysicsElectrosynthesis
Electron-deficient Ru sites at Ru/Co(OH) 2 heterointerfaces weaken the d–p orbital hybridization ability and further facilitate the desorption of ammonia intermediates, thereby achieving ultrahigh nitrate electroreduction activity towards ammonia.
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