Advanced Materials · 2019 · 45 citations · 33 references
EngineeringMaterials EngineeringMaterials ScienceOptical MaterialsPhotonicsSemiconductor DevicesDisplay TechnologiesFiber OpticsOptical FibersPhotonic MaterialsQuantum DotsQuantum OptoelectronicsCurrent EfficiencyFabricationHigh PerformanceLiquid-liquid Mass TransferLuminanceQuantum Dot DevicesQuantum Dot DisplaysQuantum Dot Light-emitting Diodes
Abstract Solution processing is widely used for preparing quantum dot (QD) films for fabricating QD light‐emitting diode display (QLED) devices. However, current approaches suffer from either the coffee‐ring effect or a large amount of wasted solution, leading to low performance and high cost. Here, a facile approach guided by a fibrous liquid bridge is developed for the continuous and controllable transfer of QD solution into ultrasmooth films by using a taut fiber with its two ends placed into capillary tubes. Guided along the fiber, a liquid bridge is formed between the horizontal fiber and the substrate, with a large mass of liquid steadily being held within the vertically placed tubes. Directionally moving the liquid bridge generates a high‐quality QD film on the substrate. Particularly, the liquid consumption is quantitative, namely, in proportion to the area of the as‐prepared film. Moreover, multilayered ultrasmooth red/green/blue QD films are prepared by multiple transfers of liquid onto the same targeted area in sequence. The as‐prepared white QLEDs show a rather high performance with a maximum luminance of 57 190 cd m −2 and a maximum current efficiency of 15.868 cd A −1 . It is envisioned that this strategy offers new perspectives for the low‐cost fabrication of high‐performance QLED devices.
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Natural Sciences, Materials Engineering, Materials Science +17