Characterization of cluster/monomer ratio in pulsed supersonic gas jets

Abstract

We determine cluster mass fraction fc(r,t) at position r within, and time t after firing, a pulsed supersonic gas jet by measuring femtosecond evolution of the jet’s refractive index by single-shot frequency domain holography. A fs pump pulse singly ionizes monomers, while quasi-statically ionizing and heating clusters to a level at which recombination remains negligible as clusters expand. Under these conditions, index evolves in two simple steps corresponding to monomer and cluster contributions, allowing recovery of fc without detailed cluster dynamic modeling. Variations of fc with t are measured.