Inhibition of Linear Absorption in Opaque Materials Using Phase-Locked Harmonic Generation

Abstract

We theoretically predict and experimentally demonstrate inhibition of linear absorption for phase and group velocity mismatched second- and third-harmonic generation in strongly absorbing materials, GaAs, in particular, at frequencies above the absorption edge. A 100-fs pump pulse tuned to 1300 nm generates 650 and 435 nm second- and third-harmonic pulses that propagate across a $450\mathrm{\text{\ensuremath{-}}}\ensuremath{\mu}\mathrm{m}$-thick GaAs substrate without being absorbed. We attribute this to a phase-locking mechanism that causes the pump to trap the harmonics and to impress on them its dispersive properties.