Nature Communications · 2022 · 58 citations · 45 references
Natural SciencesMaterials SciencePhysicsCondensed Matter PhysicsQuantum MechanicsSpectroscopyGraphene NanomaterialsMagnetic Properties Of SolidsQuantum BitsQuantum DotsRelaxation MechanismsSpintronic MaterialsElectron Relaxation DynamicsElectron Spin RelaxationRelaxation Time MeasurementsRelaxation TimesSpin QubitsSpin RelaxationSpin Relaxation DynamicsTransverse Relaxation Time
Abstract The relaxation time of a single-electron spin is an important parameter for solid-state spin qubits, as it directly limits the lifetime of the encoded information. Thanks to the low spin-orbit interaction and low hyperfine coupling, graphene and bilayer graphene (BLG) have long been considered promising platforms for spin qubits. Only recently, it has become possible to control single-electrons in BLG quantum dots (QDs) and to understand their spin-valley texture, while the relaxation dynamics have remained mostly unexplored. Here, we report spin relaxation times ( T 1 ) of single-electron states in BLG QDs. Using pulsed-gate spectroscopy, we extract relaxation times exceeding 200 μ s at a magnetic field of 1.9 T. The T 1 values show a strong dependence on the spin splitting, promising even longer T 1 at lower magnetic fields, where our measurements are limited by the signal-to-noise ratio. The relaxation times are more than two orders of magnitude larger than those previously reported for carbon-based QDs, suggesting that graphene is a potentially promising host material for scalable spin qubits.
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