Nitrogen Arylation for Macrocyclization of Unprotected Peptides

Guillaume Lautrette, Fayçal Touti, Hong Geun Lee, Peng Dai, Bradley L. Pentelute

Journal of the American Chemical Society · 2016 · 128 citations · 35 references

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Abstract

We describe an efficient and mild method for the synthesis of macrocyclic peptides via nitrogen arylation from unprotected precursors. Various electrophiles and lysine-based nucleophiles were investigated and showed high-yielding product formation, even for a macrocyclization scan with 14 variants. We found that nitrogen-linked aryl products were more stable to base and oxidation when compared to thiol arylated species, thereby highlighting the utility of this methodology. Finally, N-aryl macrocyclization was performed on a p53 peptide inhibitor of MDM2 and resulted in identification of a nanomolar binder with improved proteolytic stability and cell permeability.

References

35