Physical Review A · 2013 · 14 citations · 17 references
Natural SciencesPhysicsAtomic PhysicsQuantum MechanicsSpectroscopyAtomic ExcitationAtomic IonizationElectronic Excited StatesPhotoelectron SpectroscopyElectron Excitation ProcessesGround-state Electron ConfigurationsPeriodic MotionStrong-field IonizationStrong-field Laser-matter InteractionTime-resolved Photoelectron SpectroscopyUltrafast Electron DynamicsWave Packet Propagation
We present a real-time observation of electron motion in the ground state of the carbon atom. A wave packet is created in the ground triplet state of the atom via photodetachment of its negative ion in a strong laser field. Its dynamics is probed using the selectivity of strong-field ionization to orbital alignment in combination with an electron-imaging technique. A strong temporal modulation in the photoelectron yield at high kinetic energies is observed, which reveals a periodic motion of the electron cloud in the atom.
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Real-time observation of valence electron motion
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Electron localization following attosecond molecular photoionization
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