Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE · 2015 · 115 citations · 9 references
Natural SciencesPhysicsPhotonicsRadiation PhysicsSpectroscopyAccelerator PhysicsInfrared SpectroscopyOptical SpectroscopyTerahertz PhotonicsTerahertz SpectroscopyUltrafast OpticsElectron AcceleratorsEmittanceIon MobilityIon Mobility SpectrometryNear-infrared RadiationTerahertz GenerationTerahertz OscillatorsTerahertz Sources
A mid-infrared oscillator FEL has been commissioned at the Fritz Haber Institute. The accelerator consists of a thermionic gridded gun, a subharmonic buncher, and two S-band standing-wave copper structures. It provides a final electron energy adjustable from 15 to 50 MeV, low longitudinal (< 50 keV ps) and transverse emittance (< 20 πmm mrad), at more than 200 pC bunch charge with a micro-pulse repetition rate of 1 GHz and a macro-pulse length of up to 15 <i>µ</i>s. Pulsed radiation with up to 100 mJ macro-pulse energy at about 0.5% FWHM bandwidth is routinely produced in the wavelength range from 4 to 48 <i>µ</i>m. A characterization of the FEL performance in terms of pulse energy, bandwidth, and micro-pulse shape of the IR radiation is given. In addition, selected user results are presented. These include, for instance, spectroscopy of bio-molecules (peptides and small proteins) either conformer selected by ion mobility spectrometry or embedded in superfluid helium nano-droplets at 0.4 K, as well as vibrational spectroscopy of mass-selected metal-oxide clusters and protonated water clusters in the gas phase.
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Protomers of Benzocaine: Solvent and Permittivity Dependence
Stephan Warnke, Jongcheol Seo, Jasper Boschmans et al. · Journal of the American Chemical Society · 2015 · 221 citations · Full text
Glenn B. S. Miller, Tim K. Esser, Harald Knorke et al. · Angewandte Chemie International Edition · 2014 · 84 citations
Joseph A. Fournier, Conrad T. Wolke, Christopher J. Johnson et al. · Proceedings of the National Academy of Sciences · 2014 · 64 citations · Full text
Natural Sciences, Chemistry, Physics +17