Journal of Physics A Mathematical and General · 1984 · 70 citations · 6 references
Natural SciencesChemistryPhysicsChemical KineticsPhysical ChemistryStochastic ProcessesBrownian MotionDecay ProcessesDiffusion ProcessesDiffusion-controlled ReactionsKinetic ModelingReaction-diffusion SystemsKinetic Monte Carlo SimulationKinetic Transport EquationsMonte Carlo Particle TransportReaction-diffusion EquationsReaction-diffusion Stochastic ModelsSpatial KineticsTrap KineticsTraps
The authors study the kinetics of a diffusion-controlled reaction in which perfect traps (scavengers) diffuse and consume randomly distributed particles. They find that the number of particles remaining after time t decays as exp(- alpha ctd2/), for spatial dimensions d<2, and as exp(- alpha ct) for d>or=2, where alpha is a constant, and c is the trap concentration. These predictions are supported by Monte Carlo data in d=1 and d=2. They also discuss the differences between the scavenger reaction and the reaction of particles diffusing and being consumed by randomly distributed static traps. Finally, they treat the situation where both the particles and the traps diffuse.
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Diffusion-Controlled Reactions
Daniel F. Calef, J. M. Deutch · Annual Review of Physical Chemistry · 1983 · 392 citations
Random-walk studies of excitation trapping in crystals
G. Zumofen, A. Blumen · Chemical Physics Letters · 1982 · 125 citations
Asymptotic Solution of Interacting Walks in One Dimension
S. Redner, K. Kang · Physical Review Letters · 1983 · 79 citations