Review of Scientific Instruments · 1993 · 126 citations · 5 references
Natural SciencesMaterials SciencePhysicsOpticsPhotonicsSpectroscopyOptical SpectroscopyScattering TheoryChemical NonequilibriumCorrelation FunctionsCorrelation In Optical SystemsDynamic Light ScatteringNonequilibrium DynamicsScattering By SpheresTime ScalesTime-resolved Scattering
We have successfully implemented a method to measure intensity autocorrelation functions with a CCD camera and a fast computer. We report light scattering experiments on solutions of diffusing latex spheres in glycerol and compare our results to those obtained with a conventional hardwired electronic correlator. Averaging allows significant reduction of measurement times and makes this technique suitable for the study of systems with very long time scales. Moreover, the CCD setup allows measurement of two-time correlation functions under nonequilibrium conditions where conventional correlators which rely on time-averaging fail. The new method may offer significant advantage for low-intensity applications like x-ray correlation spectroscopy.
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Light-scattering experiments on phase-separation dynamics in binary fluid mixtures
A. Cumming, Pierre Wiltzius, Frank S. Bates et al. · Physical Review A · 1992 · 169 citations