Physical Review Letters · 2009 · 95 citations · 20 references
Natural SciencesChemistryPhysicsCondensed Matter PhysicsMolecular PhysicsSpectroscopyCold Atom PhysicsLaser CoolingStates Of MatterCold Atom SpectroscopyCold Molecule PhysicsCold Molecule SpectroscopyCryogenic CoolingLaser Cooling Of MoleculesMolecular CoolingRovibrational SpectraRovibrational Spectroscopy
We present a method which delivers a continuous, high-density beam of slow and internally cold polar molecules. In our source, warm molecules are first cooled by collisions with a cryogenic helium buffer gas. Cold molecules are then extracted by means of an electrostatic quadrupole guide. For ${\mathrm{ND}}_{3}$ the source produces fluxes up to $(7{\ifmmode\pm\else\textpm\fi{}}_{4}^{7})\ifmmode\times\else\texttimes\fi{}{10}^{10}\text{ }\text{ }\mathrm{\text{molecules}}/\mathrm{s}$ with peak densities up to $(1.0{\ifmmode\pm\else\textpm\fi{}}_{0.6}^{1.0})\ifmmode\times\else\texttimes\fi{}{10}^{9}\text{ }\text{ }\mathrm{\text{molecules}}/{\mathrm{cm}}^{3}$. For ${\mathrm{H}}_{2}\mathrm{CO}$ the population of rovibrational states is monitored by depletion spectroscopy, resulting in single-state populations up to $(82\ifmmode\pm\else\textpm\fi{}10)%$.
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Diffuse Atomic and Molecular Clouds
Theodore P. Snow, Benjamin J. McCall · Annual Review of Astronomy and Astrophysics · 2006 · 580 citations
Natural Sciences, Chemistry, Physics +17
Measurement of the Electron Electric Dipole Moment Using YbF Molecules
J. J. Hudson, B. E. Sauer, M. R. Tarbutt et al. · Physical Review Letters · 2002 · 419 citations · Full text