Journal of the American Chemical Society · 2013 · 35 citations · 38 references
Natural SciencesChemistryElectronic MaterialsOrganic ChemistryQuantum ChemistryHeterocyclic ChemistryHeterocyclic CompoundsMacrocycle SynthesisOrganic SynthesisPhotochemical SynthesisPhotochemistry[2+2] CycloadditionAlkyne Cycloaddition ReactionsCycloaddition ReactionsElectrocyclic ReactionsPhotochemical CycloadditionPhotochemical Reaction MechanismsPolycyclic Scaffold DiversificationThiophene Chemistry
A new bisdehydro[12]annulene derivative having a thiophene-fused structure has been synthesized. This highly twisted π-conjugated macrocycle with two acetylene moieties in close proximity produces a [2+2]-type alkyne cycloadduct by either photoirradiation or mild heating without any transition metals. Theoretical calculations reveal that the thermal reaction proceeds through successive 8π and 4π electrocyclic reactions, while the photochemical reaction is an asynchronous concerted [2+2] cycloaddition. The fused structure with the less-aromatic thiophene ring is crucial for achieving this reaction. The cycloadduct, thiophene-fused biphenylene, has significant potential as a new polycyclic π-scaffold for electronic applications.
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The path of chemical reactions - the IRC approach
Kenichi Fukui · Accounts of Chemical Research · 1981 · 6.6K citations