Optical Ramsey fringes with traveling waves

Abstract

We present a new interaction geometry for optical Ramsey fringes comprised of four traveling waves instead of the three usual standing waves. First, we demonstrate experimentally that the new method leads to an improved contrast, using the optothermal detection of the vibrational excitation of ${\mathrm{SF}}_{6}$ in a supersonic beam illuminated by a waveguide ${\mathrm{CO}}_{2}$ laser. Second, we give a simple theoretical description of the method, using evolution matrices of spinors and pseudospin-vector representations of these spinors. Finally, we introduce strong-field density-matrix diagrams to discuss the differences between the various interaction geometries as well as between the Ramsey fringes and the usual stimulated photon echoes.