Novel Spin Features in Raman Spectra of Few-Electron Quantum Dots

Abstract

We employ a self-consistent, dynamic spin-density functional concept beyond the dipole approximation in order to calculate the collective modes of few-electron quantum dots with partial spin polarization. Because of Hund's rule in a magnetic field the mode energies exhibit characteristic discontinuities in their magnetic-field dependence, which is a manifestation of ground-state transitions between different spin configurations. A finite ground-state spin density couples collective charge- and spin-density excitations. We predict their observability in state-of-the-art Raman experiments.