Physical Review Letters · 2012 · 130 citations · 19 references
Natural SciencesPhysicsOpticsPhotonicsSpectroscopyOptical CoherenceUltrafast OpticsX-ray OpticsBeam CoherenceBeam Pulse DurationCoherence PropertiesCoherence TimeCoherent Light SourcesColloidal NanoparticlesSingle ShotTemporal Coherence
We measured the transverse and longitudinal coherence properties of the Linac Coherent Light Source (LCLS) at SLAC in the hard x-ray regime at 9 keV photon energy on a single shot basis. Speckle patterns recorded in the forward direction from colloidal nanoparticles yielded the transverse coherence properties of the focused LCLS beam. Speckle patterns from a gold nanopowder recorded with atomic resolution allowed us to measure the shot-to-shot variations of the spectral properties of the x-ray beam. The focused beam is in the transverse direction fully coherent with a mode number close to 1. The average number of longitudinal modes behind the Si(111) monochromator is about 14.5 and the average coherence time ${\ensuremath{\tau}}_{c}=(2.0\ifmmode\pm\else\textpm\fi{}1.0)\text{ }\text{ }\mathrm{fs}$. The data suggest a mean x-ray pulse duration of $(29\ifmmode\pm\else\textpm\fi{}14)\text{ }\text{ }\mathrm{fs}$ behind the monochromator for $(100\ifmmode\pm\else\textpm\fi{}14)\text{ }\text{ }\mathrm{fs}$ long electron pulses.
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