Publication | Closed Access
Observing the Dynamics of Dipole-Mediated Energy Transport by Interaction-Enhanced Imaging
197
Citations
27
References
2013
Year
Relaxation ProcessLocalized Excited StateEngineeringMicroscopyMagnetic ResonanceExcitation Energy TransferElectronic Excited StateUltracold AtomSpatial ResolutionMolecular ImagingBiophysicsNovel Imaging MethodQuantum SciencePhysicsContinuous Spatial ProjectionElectronic Quantum StateAtomic PhysicsPhysical ChemistryImagingQuantum ChemistryDipole-mediated Energy TransportExcited State PropertySpectroscopyElectronic ImagingBiomedical ImagingApplied PhysicsMedicine
Electronically highly excited (Rydberg) atoms experience quantum state-changing interactions similar to Förster processes found in complex molecules, offering a model system to study the nature of dipole-mediated energy transport under the influence of a controlled environment. We demonstrate a nondestructive imaging method to monitor the migration of electronic excitations with high time and spatial resolution, using electromagnetically induced transparency on a background gas acting as an amplifier. The continuous spatial projection of the electronic quantum state under observation determines the many-body dynamics of the energy transport.
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