Physical Review B · 2013 · 88 citations · 46 references
Natural SciencesPhysicsCondensed Matter PhysicsCrystal StructureQuantum MechanicsElectron CorrelationNonadiabatic DynamicsQuantum DecoherenceRelaxation MechanismsSpin DynamicsCoherence DynamicsDecoherence TimeDiamond Nitrogen-vacancy CentersFree Induction DecaySpin CoherenceSpin DephasingSpin NoiseSpin Systems
We theoretically investigate spin decoherence of a single nitrogen-vacancy (NV) center in diamond. Using the spin coherent-state $P$-representation method, we simulate coherence evolution of the NV center coupled to surrounding nitrogen electron (N) spins. In the system, the strength of N-N coupling is the same order as that of NV-N coupling (the strong intrabath coupling regime). We find that spin decoherence time as well as free-induction decay of the NV center depend on the spatial configuration of N spins. Both the spin decoherence rate ($1/{T}_{2}$) and dephasing rate ($1/{T}_{2}^{*})$ of the NV center increase linearly with the concentration of the N spins. Using the $P$-representation method, we also demonstrate extracting the noise spectrum of the N spin bath. The capability to calculate the noise spectrum will provide promising pathways to suppress decoherence of spin systems in the strong intrabath coupling regime.
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