Multi‐Path Magnetic Relaxation of Mono‐Dysprosium(III) Single‐Molecule Magnet with Extremely High Barrier

Abstract

A large magnetic anisotropy was achieved around the DyIII ion, and a single-molecule magnet behavior has been observed up to 35 K for the dinuclear complex DyIII–ZnII. The magnetic relaxation occurs through three different pathways depending on the temperature and the presence of an external dc field (see scheme). Detailed facts of importance to specialist readers are published as "Supporting Information". Such documents are peer-reviewed, but not copy-edited or typeset. They are made available as submitted by the authors. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.