All-optically controlled fourth- and sixth-order fluorescence processes of Pr3+:YSO

Abstract

We report all-optically controlled fourth- and sixth-order fluorescence processes with and without splitting, in a heteronuclear-like molecule system of Pr3+:YSO both in theory and experiment. We construct the asymptote among Pr3+ ions localized at different cation vacancies. By changing the frequency detuning and power of the controlling field, fluorescence signal can be controlled to switch from an enhanced peak to a suppressed dip, and vice versa. Such transition has a potential application to produce all-optical switches. The results can be well explained by a theory model based on the high-order coherent process.