Spectroscopy of cooperative laser electron-γ-nuclear processes in polyatomic molecules

Abstract

The consistent quantum approach to calculating the electron-nuclear γ transition spectra (a set of the vibration-rotational satellites in a molecule) of a nucleus in polyatomic molecules is used to determine accurate data of the vibration-nuclear transition probabilities. We present results for emission and absorption γ-spectra of nucleus 191Ir (E(0)γ= 82 keV) in the molecule of IrO4.