Due to their unique tubular and spiral structure, graphene and graphene oxide nanoscrolls (GONS) have shown extensive applications in various fields. However, it is still a challenge to improve the optoelectronic application of graphene and GONS because of the zero bandgap of graphene. Herein, ammonium tetrathiomolybdate ((NH₄)₂MoS₄) was firstly wrapped into the ((NH₄)₂MoS₄@GONS) by molecular combing the mixture of (NH₄)₂MoS₄ and GO solution on hydrophobic substrate. After thermal annealing, the (NH₄)₂MoS₄ and GO were converted to MoS₂ nanosheets and reduced GO (RGO) simultaneously, and, thus, the MoS₂@RGONS was obtained. Raman spectroscopy and high-resolution transmission electron microscopy were used to confirm the formation of MoS₂ nanosheets among the RGONS. The amount of MoS₂ wrapped in RGONS increased with the increasing height of GONS, which is confirmed by the atomic force microscopy and Raman spectroscopy. The as-prepared MoS₂@RGONS showed much better photoresponse than the RGONS under visible light. The photocurrent-to-dark current ratios of photodetectors based on MoS₂@RGONS are ~570, 360 and 140 under blue, red and green lasers, respectively, which are 81, 144 and 35 times of the photodetectors based on RGONS. Moreover, the MoS₂@RGONS-based photodetector exhibited good power-dependent photoresponse. Our work indicates that the MoS₂@RGONS is expected to be a promising material in the fields of optoelectronic devices and flexible electronics.

#	Concept	H-Index	Publications	Citations
1	Engineering	2	2	62
2	Chemical Engineering	2	2	62
3	Chemistry	2	2	62
4	Applied Physics	1	1	21
5	Environmental Engineering	1	1	41

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