1b:I[76749,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"default"] 1c:I[3486,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"default"] 1d:I[41892,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"default"] 1e:I[17707,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"default"] 1f:I[66528,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"default"] 20:I[63176,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"default"] 21:I[87099,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"default"] 22:I[26200,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"Group"] 23:I[23365,["/_next/static/chunks/f9f65a69b09cd00d.js","/_next/static/chunks/1ba21a8e081e29d1.js","/_next/static/chunks/0383663887945ae7.js","/_next/static/chunks/5bf36002c846d2d8.js","/_next/static/chunks/63561dcd578bd4db.js","/_next/static/chunks/29d2646804fd1cab.js","/_next/static/chunks/2060b26370dc6c0a.js"],"default"] 24:T43e,This paper reports an approach to repurpose low-cost, bulk multilayer MoS₂ for development of ultraefficient hydrogen evolution reaction (HER) catalysts over large areas (>cm²). We create working electrodes for use in HER by dry transfer of MoS₂ nano- and microflakes to gold thin films deposited on prestrained thermoplastic substrates. By relieving the prestrain at a macroscopic scale, a tunable level of tensile strain is developed in the MoS₂ and consequently results in a local phase transition as a result of spontaneously formed surface wrinkles. Using electrochemical impedance spectroscopy, we verified that electrochemical activation of the strained MoS₂ lowered the charge transfer resistance within the materials system, achieving HER activity comparable to platinum (Pt). Raman and X-ray photoelectron spectroscopy show that desulfurization in the multilayer MoS₂ was promoted by the phase transition; the combined effect of desulfurization and the lower charge resistance induced superior HER performance.

Dohyun Rhuy

Publications