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Evidence for Low-Intensity D-D Reaction as a Result of Exothermic Deuterium Desorption from Au/Pd/PdO:D Heterostructure
26
Citations
14
References
2000
Year
Low-intensity Nuclear EmissionsEngineeringNuclear PhysicsNuclear DataChemistryNe213 Neutron DetectionChemical EngineeringNuclear MaterialsHigh-energy Nuclear ReactionRadiation DetectionPhysicsAccelerator Mass SpectrometryLow-intensity D-d ReactionNuclear TheoryNeutron SourceAtomic PhysicsDeuterium DesorptionPhysical ChemistryCatalysisHydrogenExperimental Nuclear PhysicsD HeterostructureNatural SciencesDetector PhysicNuclear ExperimentsExothermic Deuterium DesorptionChemical Kinetics
Low-intensity nuclear emissions (neutrons and charged particles) due to exothermic deuterium desorption from Au/Pd/PdO heterostructure loaded with deuterium by electrolysis have been studied by NE213 neutron detection as well as SSB and CR-39 charged-particle detectors in low-background conditions with large statistics. Similar measurements were performed with the Au/Pd/PdO:H heterostructure as a control. It has been established that in experiments with the Au/Pd/PdO:D system, the excessive 2.45-MeV neutrons and 3.0-MeV protons are better detected than with the Au/Pd/PdO:H system, where those detection rates for n and p did not exceed the cosmic background level. The levels of neutron and proton emissions for 40- to 60-μm-thick samples are found to be close to one another and after subtracting background (Au/Pd/PdO:H count rate) consist of In = (19 ± 2)·10-3 n/s and Ip = (4.0 ± 1.0)·10-3 p/s in a 4π solid angle, respectively. These yields of D-D reaction products in Au/Pd/PdO heterostructure comply with the mean D-D reaction rate of λdd ~ 10-23s-1 per D-D pair.
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