1e:T49b,Conductive hydrogels have shown great promise in flexible electronics, but their practical applications may be impeded by the time-consuming and energy-consuming polymerization process. We proposed a sodium lignosulfonate-Fe (SLS-Fe) strategy to address this challenge and took advantage of carboxymethyl cellulose (CMC) and poly(acrylic acid) to prepare the CMC/PAA/Fe³⁺/LiCl interpenetrating conductive hydrogels with good self-healing properties, antifreezing properties, and a 6-fold increase in conductivity in this study. The hydrogel-based flexible strain sensors demonstrated a broad detection range (400%), high sensitivity (GF = 6.19 at 200-400%), and human motion detection capability. The hydrogel-based supercapacitor exhibited a single-electrode specific capacitance of 122.36 F g^-1 which successfully powered LEDs. Furthermore, the supercapacitor showed a single-electrode specific capacitance of 83.16 F g^-1 at -23 °C (68% of the one exhibited at 25 °C). Therefore, the multifunctional performance of the CMC/PAA/Fe³⁺/LiCl hydrogel is anticipated to play an exemplary role in a new generation of flexible electronics.1f:T45e,Recently, the health problems faced by sedentary workers have received increasing attention. In this study, a pressure sensor based on a poly(dimethylsiloxane) (PDMS)/carboxylated chitosan (CCS)/carboxylated multiwalled carbon nanotube (cMWCNT) sponge was prepared to realize a portable, sensitive, comfortable, and noninvasive healthcare monitoring system for sedentary workers. The proposed piezoresistive pressure sensor exhibited exceptional sensing performances with high sensitivity (147.74 kPa^-1), an ultrawide detection range (22 Pa to 1.42 MPa), and reliable stability (over 3000 cycles). Furthermore, the obtained sensor displayed superior capability in detecting various human motion signals. Based on the 4 × 4 sensing array and multilayer perceptron (MLP) algorithm model, a smart cushion was developed to recognize five types of sitting postures and supply timely reminders to sedentary workers. The piezoresistive sponge pressure sensor proposed in this study reveals promising potential in the fields of wearable electronics, healthcare monitoring, and human-machine interface applications.

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