Nature Communications · 2024 · 59 citations · 44 references
Natural SciencesMaterials EngineeringMaterials ScienceNanotechnologyOptical MaterialsPhotonicsDielectricsElectro-optic EffectsElectro-optic MaterialsOptical PolymersOptical ResonatorsPhotonic MaterialsDielectric ConstantElectro-optic PolymersMetamaterialsMetasurfacesPlanar ResonatorsSymmetry ControlTunable Optical ResonatorsTunable Photonic Devices
Achieving precise spectral and temporal light manipulation at the nanoscale remains a critical challenge in nanophotonics. While photonic bound states in the continuum (BICs) have emerged as a powerful means of controlling light, their reliance on geometrical symmetry breaking for obtaining tailored resonances makes them highly susceptible to fabrication imperfections, and their generally fixed asymmetry factor fundamentally limits applications in reconfigurable metasurfaces. Here, we introduce the concept of environmental symmetry breaking by embedding identical resonators into a surrounding medium with carefully placed regions of contrasting refractive indexes, activating permittivity-driven quasi-BIC resonances (ε-qBICs) without altering the underlying resonator geometry and unlocking an additional degree of freedom for light manipulation through active tuning of the surrounding dielectric environment. We demonstrate this concept by integrating polyaniline (PANI), an electro-optically active polymer, to achieve electrically reconfigurable ε-qBICs. This integration not only demonstrates rapid switching speeds and exceptional durability but also boosts the system's optical response to environmental perturbations. Our strategy significantly expands the capabilities of resonant light manipulation through permittivity modulation, opening avenues for on-chip optical devices, advanced sensing, and beyond.
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Natural Sciences, Materials Engineering, Materials Science +17