Cell Reports Physical Science · 2024 · 48 citations · 45 references
EngineeringMaterials ScienceAgingElectrochemical EngineeringPredictive AnalyticsBattery MaterialsBattery SystemsBattery TechnologyBattery TestingEnergy StorageLongevityBattery AgingBattery DegradationBattery ModelingDegradationHierarchical Bayesian ModelLifetime EstimationLifetime PredictionLithium-ion Batteries
Accurate battery lifetime prediction is important for maintenance, warranties, and cell design, but manufacturing variability and usage‑dependent degradation make it challenging. We investigate new features derived from early‑life capacity‑voltage data to predict the lifetime of cells cycled under varying charge rates, discharge rates, and depths of discharge. We use early‑life capacity‑voltage features that capture a cell's state of health and the change rate of component‑level degradation modes to predict lifetime under varying cycling conditions. Using a dataset of 225 Ni‑Mn‑Co/graphite cells, we achieve 15.1 % MAPE on in‑distribution predictions and 21.8 % MAPE on out‑of‑distribution predictions, demonstrating that domain‑knowledge‑informed feature engineering and a hierarchical Bayesian model improve lifetime prediction, and we provide a new publicly available aging dataset.
Accurate battery lifetime prediction is important for maintenance, warranties, and cell design. However, manufacturing variability and usage-dependent degradation make life prediction challenging. Here, we investigate new features derived from capacity-voltage data in early life to predict the lifetime of cells cycled under varying charge rates, discharge rates, and depths of discharge. The early-life features capture a cell's state of health and the change rate of component-level degradation modes. Using a newly generated dataset from 225 nickel-manganese-cobalt/graphite lithium-ion cells aged under a wide range of conditions, we demonstrate a lifetime prediction of in-distribution cells with 15.1% mean absolute percentage error (MAPE). A hierarchical Bayesian model shows improved performance on extrapolation, achieving 21.8% MAPE for out-of-distribution cells. Our approach highlights the importance of using domain knowledge of battery degradation to inform feature engineering and model construction. Further, a new publicly available battery lifelong aging dataset is provided.
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