Density-discriminating chromatic x-ray imaging based on metal halide nanocrystal scintillators

Abstract

X-ray imaging based on a single gray level shows visual blind parts and affects accurate judgment in some situations. Color-cognized x-ray imaging will boost the recognition capability, which has not yet been reported. Here, we propose a quartz-assisted chromatic x-ray imaging model based on metal halide nanocrystal (NC) stacked scintillators. Mutually inactive (BA) 2 PbBr 4 :Mn and Cs 3 Cu 2 I 5 :Tl enable x-ray energy- or density-dependent radioluminescence (RL) color variation. The upper scintillator light yield and the bottom scintillator transmittance are enhanced by elaborate in situ passivation of phenethylamine bromide and NC orientation regulation, respectively. Imaging targets with different densities are distinguished on RL spectra, and the color coordinates shift linearly on CIE 1931. An algorithm balances the image details of different gray areas and enhances the visual perception by color filling. This work provides color recognition between objects with different densities and takes a step toward chromatic x-ray imaging applied to practical scenarios.