Advanced Energy Materials · 2023 · 94 citations · 40 references
Natural SciencesChemical EngineeringChemistryCatalysisElectrochemistryReaction EngineeringCatalyst DesignElectrochemical CellsElectrochemical Energy ConversionElectrochemical SynthesisElectrode-electrolyte InterfacesElectrolysis ProcessesCurrent DensityElectrocatalyst DesignElectrocatalystsMultiphase ChemistryStructured CatalystsSupported ElectrocatalystsTip Interaction
Abstract N 2 and CO 2 fixation is an environmentally friendly waste‐to‐energy technology that can replace tedious and demanding industrial urea productive processes. Here, V N ‐Cu 3 N‐300 catalysts with tip and vacancy structures are designed for the coactivation of multiphase reactants in the urea electrosynthesis process. Under environmental conditions, the urea yield is 81 µg h −1 cm −2 , this is the first report of high area active electrocatalyst, and the corresponding Faraday efficiency is able to reach 28.7%. The full‐cell electrolysis exhibits good stability, providing a current density of 0.7 mA cm −2 at 2.1 V. The electrolyte after continuous electrolysis for 48 h is subjected to being evaporated and recrystallized, and it is determined by 1 H NMR that the purity of urea can reach 100%. Comprehensive analysis shows that the local electric field formed by the tip effect can effectively promote the adsorption and activation of CO 2 . The presence of surface nitrogen vacancies promotes the formation of *NN* intermediates, ensuring CN coupling, and also optimizing the dissociation process of water, providing a proton supply for the synthesis of urea. Thus, the rate‐determining step is altered and the formation of urea is ensured.
40
Molecular tuning of CO2-to-ethylene conversion
Fengwang Li, Arnaud Thevenon, Alonso Rosas‐Hernández et al. · Nature · 2019 · 1.3K citations · Full text
Coupling N2 and CO2 in H2O to synthesize urea under ambient conditions
Chen Chen, Xiaorong Zhu, Xiaojian Wen et al. · Nature Chemistry · 2020 · 1.1K citations · Full text