Advanced Optical Materials · 2023 · 15 citations · 32 references
Natural SciencesMaterials SciencePhysicsNanotechnologyOpticsPhotonicsNonlinear OpticsPhotonic MaterialsPlasmonic MaterialsPlasmonic NanomaterialsPlasmonicsRefractive IndexExtinction RatioMetamaterialsMetasurfacesModulation DepthNonlinear Optical SusceptibilityNonlinear SusceptibilityOptical NonlinearitySpatial Light Modulators
Abstract Effectual free‐space optical metasurface is essential for telecommunication and information processing. However, the lack of efficient optical nonlinearity is still an obstacle to empower its full capability and practical applications. Metallic quantum wells (MQWs) with large nonlinear susceptibility may pave a new way. Here, such MQWs are implemented into a resonance configuration of the quasi bound state in the continuum (BIC) and an efficient tunable plasmonic metasurface is proposed. Such metasurface is composed of MQWs‐based nanostructure, which supports the tunable plasmonic quasi‐BIC. The tunability is controlled through substantial change in refractive index of MQWs induced by Kerr‐type nonlinearity, which leads to around 9 dB extinction ratio and extremely high modulation speed up to terahertz level. The quasi‐BIC with narrow linewidth is obtained through symmetry‐breaking of nanoelliptical elements, further enhancing the modulation depth. This work satisfies the ultrafast‐speed and high‐efficiency requirement of free‐space all‐optical metasurfaces, including the spatial light modulators in optical computing field.
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