Proceedings of the National Academy of Sciences · 2022 · 17 citations · 30 references
Natural SciencesMaterials SciencePhysicsCondensed Matter PhysicsElectromagneticsQuantum MechanicsOptical Properties Of SolidsPlasmonic MaterialsPlasmonicsStrongly Correlated Electron SystemsSuperconducting MaterialsTerahertz SpectroscopyCoherent StatesInversion SymmetryJosephson JunctionsSpontaneous EmissionSuperconductivity In Low-dimensional SystemsSurface PlasmonsSymmetry InversionTerahertz Waves
The interplay between charge order and superconductivity remains one of the central themes of research in quantum materials. In the case of cuprates, the coupling between striped charge fluctuations and local electromagnetic fields is especially important, as it affects transport properties, coherence, and dimensionality of superconducting correlations. Here, we study the emission of coherent terahertz radiation in single-layer cuprates of the La 2-x Ba x CuO 4 family, for which this effect is expected to be forbidden by symmetry. We find that emission vanishes for compounds in which the stripes are quasi-static but is activated when c -axis inversion symmetry is broken by incommensurate or fluctuating charge stripes, such as in La 1.905 Ba 0.095 CuO 4 and in La 1.845 Ba 0.155 CuO 4 . In this case, terahertz radiation is emitted by surface Josephson plasmons, which are generally dark modes, but couple to free space electromagnetic radiation because of the stripe modulation.
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