Science · 2022 · 138 citations · 44 references
EngineeringElectrical EngineeringMaterials ScienceElectronic MaterialsNanotechnologySemiconductor DevicesNanoelectronicsNeural Circuit ModelingConductanceDynamic RangeEnergy PerformanceInterfacial Electric FieldsIonic TransportIonic Transport MechanismsIonic-electronic TransportNeuromorphic Hardware
Nanoscale ionic programmable resistors for analog deep learning are 1000 times smaller than biological cells, but it is not yet clear how much faster they can be relative to neurons and synapses. Scaling analyses of ionic transport and charge-transfer reaction rates point to operation in the nonlinear regime, where extreme electric fields are present within the solid electrolyte and its interfaces. In this work, we generated silicon-compatible nanoscale protonic programmable resistors with highly desirable characteristics under extreme electric fields. This operation regime enabled controlled shuttling and intercalation of protons in nanoseconds at room temperature in an energy-efficient manner. The devices showed symmetric, linear, and reversible modulation characteristics with many conductance states covering a 20× dynamic range. Thus, the space-time-energy performance of the all-solid-state artificial synapses can greatly exceed that of their biological counterparts.
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“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Liumin Suo, Oleg Borodin, Tao Gao et al. · Science · 2015 · 3.7K citations
Language Models are Few-Shot Learners
T. B. Brown, Benjamin Mann, Nick Ryder et al. · arXiv (Cornell University) · 2020 · 3K citations · Full text
Interface Stability in Solid-State Batteries
William D. Richards, Lincoln J. Miara, Yan Wang et al. · Chemistry of Materials · 2015 · 1.6K citations · Full text