Creep Mechanics of Epoxy Vitrimer Materials

Amber M. Hubbard, Yixin Ren, Catalin R. Picu, Alireza S. Sarvestani, Dominik Konkolewicz, Ajit K. Roy, Vikas Varshney, Dhriti Nepal

ACS Applied Polymer Materials · 2022 · 71 citations · 54 references

Concepts

TL;DR

Epoxy polymers are prized for strength and heat resistance yet are non‑recyclable and prone to fatigue and creep, driving research into vitrimer variants that employ dynamic covalent bonds for self‑healing and recyclability. This study investigates the creep behavior of epoxy vitrimers to uncover the mechanisms that cause creep and inform the design of more creep‑resistant vitrimer materials. Isothermal creep tests identify three regimes—primary chain‑mobility, secondary network rearrangement, and tertiary reaction‑error—where low temperatures behave like conventional epoxy, while high temperatures and catalyst concentrations markedly increase creep, strongly linked to catalyst level, heating rate, and temperature.

Abstract

Epoxy materials are an indispensable class of polymers due to their excellent mechanical properties and high thermal resistance. However, traditional epoxy materials are typically non-recyclable and face issues with fatigue and creep. To combat the issue of recyclability, research interest is increasingly centered on epoxy vitrimer materials, which exhibit a dynamic covalent bond exchange reaction at high temperatures allowing for self-healing, recycling, and shape reprogramming. Herein, we discuss the creep mechanics of epoxy vitrimers; we postulate that gaining a fundamental understanding of what causes creep in vitrimers will garner advances in vitrimer creep resistance for future applications. Isothermal creep results demonstrate the presence of three distinct creep regimes: primary creep associated with polymer chain mobility, secondary creep associated with network rearrangement due to the dynamic covalent bond exchange reaction, and tertiary creep associated with errors in this reaction. We note at low temperatures (T ≪ Tv) and catalyst concentrations, vitrimers simply behave as a traditional epoxy material. In contrast, at high temperatures and catalyst concentrations, vitrimers exhibit significantly more creep with strong correlations to catalyst concentration, heating rate, and temperature, which are quantified in this work.

References

54