Proceedings of the National Academy of Sciences · 2022 · 38 citations · 43 references
Natural SciencesMaterials SciencePhysicsCondensed Matter PhysicsMaterials PhysicsMaterials ThermodynamicsMetastable PhasesStatistical MechanicsFree Energy MinimizationJammingJamming TransitionsLocal Energy MinimaMetastable RegionMetastable State ThermodynamicsMetastable StatesTraining Protocols
SignificanceMany protocols used in material design and training have a common theme: they introduce new degrees of freedom, often by relaxing away existing constraints, and then evolve these degrees of freedom based on a rule that leads the material to a desired state at which point these new degrees of freedom are frozen out. By creating a unifying framework for these protocols, we can now understand that some protocols work better than others because the choice of new degrees of freedom matters. For instance, introducing particle sizes as degrees of freedom to the minimization of a jammed particle packing can lead to a highly stable state, whereas particle stiffnesses do not have nearly the same impact.
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Supercooled Liquids and Glasses
M. D. Ediger, C. A. Angell, Sidney R. Nagel · The Journal of Physical Chemistry · 1996 · 2.2K citations
Structural Relaxation Made Simple
Erik Bitzek, Pekka Koskinen, Franz Gähler et al. · Physical Review Letters · 2006 · 1.7K citations
Organic Glasses with Exceptional Thermodynamic and Kinetic Stability
Stephen F. Swallen, Kenneth L. Kearns, Marie K. Mapes et al. · Science · 2006 · 788 citations
Natural Sciences, Materials Engineering, Materials Science +12