Direct Observation of Strong Anomalous Hall Effect and Proximity‐Induced Ferromagnetic State in SrIrO₃

Abstract

The 5d iridium-based transition metal oxides have gained broad interest because of their strong spin-orbit coupling, which favors new or exotic quantum electronic states. On the other hand, they rarely exhibit more mainstream orders like ferromagnetism due to generally weak electron-electron correlation strength. Here, a proximity-induced ferromagnetic (FM) state with T_C ≈ 100 K and strong magnetocrystalline anisotropy is shown in a SrIrO₃ (SIO) heterostructure via interfacial charge transfer by using a ferromagnetic insulator in contact with SIO. Electrical transport allows to selectively probe the FM state of the SIO layer and the direct observation of a strong, intrinsic, and positive anomalous Hall effect (AHE). For T ≤ 20 K, the AHE displays unusually large coercive and saturation field, a fingerprint of a strong pseudospin-lattice coupling. A Hall angle, σ_xy ^AHE /σ_xx _, larger by an order of magnitude than in typical 3d metals and an FM net moment of about 0.1 μ_B /Ir, is reported. This emphasizes how efficiently the nontrivial topological band properties of SIO can be manipulated by structural modifications and the exchange interaction with 3d TMOs.