Angewandte Chemie International Edition · 2017 · 84 citations · 57 references
Natural SciencesChemistryCatalysisDrug DiscoveryOrganic ChemistryCatalyst DesignCatalyst PreparationCatalyst SynthesisCatalytic MechanismsHeterocycle SynthesisHeterocyclic ChemistryAsymmetric CatalysisAsymmetric Catalyst DesignAsymmetric Heterocycle SynthesisBifunctional CatalysisBifunctional CatalystsCatalyst Structure - Activity RelationshipsHeterocycle FunctionalizationReactivity
Abstract N‐Boc ketimines derived from pyrazolin‐5‐ones were explored to develop an unprecedented domino aza‐Friedel–Crafts/N,O‐acetalization reaction with 2‐naphthols. The novel method requires a catalyst loading of only 0.5 mol % of a bifunctional squaramide catalyst, is scalable to gram amounts, and provides a new series of furanonaphthopyrazolidinone derivatives bearing two vicinal tetra‐substituted stereogenic centers in excellent yields (95–98 %) and stereoselectivity (>99:1 d.r. and 97–98 % ee ). A different reactivity was observed in the case of 1‐naphthols and other electron‐rich phenols, which led to the aza‐Friedel–Crafts adducts in 70–98 % yield and 47–98 % ee .
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