Chemical tuning of spin clock transitions in molecular monomers based on nuclear spin-free Ni(<scp>ii</scp>)

Abstract

the modification of the ligand shell that determines the crystal field and the magnetic anisotropy. These properties are crucial to realize model spin qubits that combine the necessary resilience against decoherence, a proper interfacing with other qubits and with the control circuitry and the ability to initialize them by cooling.