Elastoplasticity Mediates Dynamical Heterogeneity Below the Mode Coupling Temperature

Rahul Chacko, François P. Landes, Giulio Biroli, Olivier Dauchot, Andrea J. Liu, David R. Reichman

Physical Review Letters · 2021 · 48 citations · 43 references

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Abstract

As liquids approach the glass transition temperature, dynamical heterogeneity emerges as a crucial universal feature of their behavior. Dynamic facilitation, where local motion triggers further motion nearby, plays a major role in this phenomenon. Here we show that long-ranged, elastically mediated facilitation appears below the mode coupling temperature, adding to the short-range component present at all temperatures. Our results suggest deep connections between the supercooled liquid and glass states, and pave the way for a deeper understanding of dynamical heterogeneity in glassy systems.

References

43