Muscle Fibers Inspired High‐Performance Piezoelectric Textiles for Wearable Physiological Monitoring

TLDR

Next‑generation wearable biosensors that are highly biocompatible, stretchable, and robust are expected to shift healthcare from reactive, disease‑centric models to personalized prevention and health promotion. The authors develop a muscle‑fiber‑inspired nonwoven piezoelectric textile with tunable mechanical properties for wearable physiological monitoring. Polydopamine is dispersed into electrospun BTO/PVDF nanofibers to mimic muscle fibers, improving interfacial adhesion, mechanical strength, and piezoelectric performance. Experimental and phase‑field simulations confirm enhanced mechanical and piezoelectric properties, and the resulting lightweight textile achieves 3.95 V N⁻¹ sensitivity, <3 % decline after 7,400 cycles, and supports pulse‑wave measurement, motion monitoring, and voice recognition, offering a cost‑effective, self‑powered wearable for personalized healthcare.

Abstract

Abstract The next‐generation wearable biosensors with highly biocompatible, stretchable, and robust features are expected to enable the change of the current reactive and disease‐centric healthcare system to a personalized model with a focus on disease prevention and health promotion. Herein, a muscle‐fiber‐inspired nonwoven piezoelectric textile with tunable mechanical properties for wearable physiological monitoring is developed. To mimic the muscle fibers, polydopamine (PDA) is dispersed into the electrospun barium titanate/polyvinylidene fluoride (BTO/PVDF) nanofibers to enhance the interfacial‐adhesion, mechanical strength, and piezoelectric properties. Such improvements are both experimentally observed via mechanical characterization and theoretically verified by the phase‐field simulation. Taking the PDA@BTO/PVDF nanofibers as the building blocks, a nonwoven light‐weight piezoelectric textile is fabricated, which hold an outstanding sensitivity (3.95 V N −1 ) and long‐term stability (&lt;3% decline after 7,400 cycles). The piezoelectric textile demonstrates multiple potential applications, including pulse wave measurement, human motion monitoring, and active voice recognition. By creatively mimicking the muscle fibers, this work paves a cost‐effective way to develop high‐performance and self‐powered wearable bioelectronics for personalized healthcare.