Nonlinear Bound States in the Continuum of Etchless Lithium Niobate Metasurfaces

Abstract

Optical bound states in the continuum (BICs) have recently been studied in a wide range of material systems, where light is perfectly confined in the continuous spectrum of radiating modes. In this paper, we reported periodic nonlinear metasurfaces on the etchless LiNbO <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> platform, realizing the enhancement of second-order generation (SHG). All-dielectric heterogeneous metasurfaces are constructed by patterning a low-refractive-index polymer on a high refractive-index LiNbO <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> film without etching. Due to BICs, light is localized in the LiNbO <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> film where the excellent optical second-order nonlinearity is exploited. We demonstrated that with normal incident waves, symmetry-protected BICs are formed at near-infrared wavelength showing a vanishing linewidth in the transmission spectrum. In addition, to manifest the invisible BICs to detectable supercavity resonances at normal incidence, asymmetry is introduced into the system, degrading the symmetry-protected BICs to sharp resonances with a high Q factor. Furthermore, the second harmonic generation (SHG) of the etchless lithium niobate metasurface is studied, predicting that the SHG efficiency can exceed 10 <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">-3</sup> with 30 MW/cm <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</sup> of the pump intensity. The proposed strategy without facing the fabrication challenge of etching single-crystal LiNbO <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> film opens a new avenue for the utilization of BIC in nonlinear optics of all-dielectric heterogeneous metasurfaces.