Angewandte Chemie International Edition · 2019 · 126 citations · 29 references
Natural SciencesChemistryCatalysisOrganic ChemistryReaction EngineeringPhotocatalysisPhotochemical SynthesisPhotochemistryMild Reaction ConditionsOrganic Molecule SynthesisPhotocatalytic SynthesisPhotochemical EffectsPhotochemical FunctionalizationPhotochemical ProcessesPhotochemical Reaction MechanismsPhotochemical Reactions
Hexafluoroisopropanol is typically considered as an unreactive solvent and not as a reagent in organic synthesis. Herein, we report on a mild and efficient photochemical reaction of aryl diazoacetates with hexafluoroisopropanol that enables, under stoichiometric reaction conditions, the synthesis of fluorinated ethers in excellent yield. Mechanistic studies indicate there is a preorganization of hexafluoroisopropanol and the diazoalkane acts as an unreactive hydrogen-bonding complex. Only after photoexcitation does this complex undergo a protonation-substitution reaction to the reaction product. Investigations on the applicability of this photochemical transformation show that a broad variety of acidic alcohols can be subjected to this transformation and thus demonstrate the feasibility of this concept for O-H functionalization reactions (54 examples, up to 98 % yield).
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Blue light-promoted photolysis of aryldiazoacetates
Igor D. Jurberg, Huw M. L. Davies · Chemical Science · 2018 · 395 citations · Full text
Enantioselective iron-catalysed O–H bond insertions
Shou‐Fei Zhu, Yan Cai, Hong‐Xiang Mao et al. · Nature Chemistry · 2010 · 271 citations