Geophysical Research Letters · 2019 · 47 citations · 34 references
Natural SciencesEarth SciencesEnvironmental SciencesAir PollutionAtmospheric ChemistryAtmospheric ScienceAir Pollutant EmissionsAir PollutantsAir Pollution ModelingAir QualityAtmospheric Composition ChangeEmission InventoriesAir Pollutant InventoriesBayesian InversionEmission EstimationEmission Inventory AnalysisEmission ModelsEmissions Inventory DataParticle DispersionParticle Dispersion Modeling
Abstract Hydrochlorofluorocarbons (HCFCs), the main substitutes of chlorofluorocarbons, are regulated by the Montreal Protocol. Chinese HCFC emissions increased fast from the beginning of this century. However, limit reports based on atmospheric measurement are available for years after 2011, an important period when significant changes are expected. Combining atmospheric observations at seven sites across China with a FLEXible PARTicle dispersion model‐based Bayesian inversion technique, we estimate emission magnitudes and changes of four major HCFCs in China during 2011–2017. The emissions of all four HCFCs reached peaks before 2015. Our results agreed well with the reported bottom‐up inventories. The Chinese ozone depletion potential (ODP)‐weighted emission of the three most abundant HCFCs accounted for 37% of global totals from 2011 to 2016. The total emission of HCFC‐22 from China, the European Union, and the United States accounted approximately a half of the global totals, suggesting large HCFC emission emitted from the rest of the world.
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B. R. Miller, Ray F. Weiss, Peter K. Salameh et al. · Analytical Chemistry · 2008 · 376 citations
A. Stohl, Petra Seibert, Jgor Arduini et al. · Atmospheric chemistry and physics · 2009 · 281 citations · Full text
Natural Sciences, Earth Sciences, Environmental Sciences +17