Physical review. B./Physical review. B · 2019 · 49 citations · 34 references
Natural SciencesMaterials SciencePhysicsElectronic MaterialsMaterials PhysicsOptical MaterialsElectro-optic EffectsElectro-optic MaterialsElectronic Band StructureInfrared Optical MaterialsInfrared SpectroscopyOptical Properties Of SolidsBand Structure EngineeringGrapheneInfrared TransmissionInfrared Transmission PropertiesOptical AbsorptionOptical Absorption SpectraOptical Properties Of GraphenePhotonic Band Structure
We report the infrared transmission measurement on electrically gated twisted bilayer graphene. The optical absorption spectrum clearly manifests dramatic changes such as the splitting of the interlinear-band absorption step, the shift of the inter-van Hove singularity transition peak, and the emergence of a very strong intravalence (intraconduction) band transition. These anomalous optical behaviors demonstrate consistently a nonrigid band structure modification created by ion-gel gating through layer-dependent Coulomb screening. We propose that this screening-driven band modification is a universal phenomenon that persists to other bilayer crystals in general, establishing electrical gating as a versatile technique to engineer band structures and to create different types of optical absorptions that can be exploited in electro-optical device applications.
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