Angewandte Chemie International Edition · 2018 · 658 citations · 44 references
Natural SciencesChemical EngineeringChemistryCatalysisMaterials ChemistryReaction EngineeringCatalyst DesignCatalyst PreparationCatalyst SynthesisCatalytic MaterialsIndustrial CatalysisRedox-active MaterialsActive SitesCatalyst Active SitesFaradaic EfficiencyNitrogen-doped CarbonNon-precious Metal CatalystsPorous CarbonSingle-atom Catalyst DesignSingle-atom Catalysts
Abstract NH 3 synthesis by the electrocatalytic N 2 reduction reaction (NRR) under ambient conditions is an appealing alternative to the currently employed industrial method—the Haber–Bosch process—that requires high temperature and pressure. We report single Mo atoms anchored to nitrogen‐doped porous carbon as a cost‐effective catalyst for the NRR. Benefiting from the optimally high density of active sites and hierarchically porous carbon frameworks, this catalyst achieves a high NH 3 yield rate (34.0±3.6 μg h −1 mg cat. −1 ) and a high Faradaic efficiency (14.6±1.6 %) in 0.1 m KOH at room temperature. These values are considerably higher compared to previously reported non‐precious‐metal electrocatalysts. Moreover, this catalyst displays no obvious current drop during a 50 000 s NRR, and high activity and durability are achieved in 0.1 m HCl. The findings provide a promising lead for the design of efficient and robust single‐atom non‐precious‐metal catalysts for the electrocatalytic NRR.
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Ning Zhang, Abdul Jalil, Daoxiong Wu et al. · Journal of the American Chemical Society · 2018 · 992 citations