Unidirectional Enhanced Emission from 2D Monolayer Suspended by Dielectric Pillar Array

Abstract

Monolayers of transition metal dichalcogenides show great promise for optoelectronic devices as atomically thin semiconductors. Although dielectric or metal nanostructures have been extensively studied for tailoring and enhancing emission from monolayers, their applications are limited because of the mode concentrating inside the dielectric or the high optical losses in metals, together with the low quantum yield in monolayers. Here, we demonstrate that a metal-backed dielectric pillar array can suspend monolayers to increase the radiative recombination, and simultaneously, create strongly confined band-edge modes on surface directly accessible to monolayers. We observe unidirectional enhanced emission from WSe 2 monolayers on polymer pillar array.