Low-threshold parametric oscillation in organically modified microcavities

Abstract

microcavities with monomolecular layers of highly nonlinear small molecules. The functionalized microcavities demonstrate high-efficiency parametric oscillation in the near-IR and generate primary frequency combs with 0.88-mW thresholds, improving optical parametric oscillation generation over nonfunctionalized devices by three orders of magnitude. This organic-inorganic approach enables otherwise unattainable performance and will inspire the next generation of integrated photonic device platforms.